Can You Convert a PS2 ISO to Play on PS1? No – Fundamental Hardware Differences
No. Direct conversion is impossible due to fundamental hardware differences.
Why It Won't Work
Architecture: PS2 uses the "Emotion Engine" (MIPS III 128-bit, 299 MHz) + Vector Units. PS1 uses a MIPS R3000A (32-bit, 33.8 MHz). PS2 games are compiled for completely different instruction sets and co-processors.
Media & File System: PS2 uses DVD-ROM (4.7 GB) with a complex file system. PS1 uses CD-ROM (650 MB) with a simpler ISO9660 structure. A PS2 ISO exceeds PS1 disc capacity and uses DVD-specific addressing.
Graphics/Audio: PS2's Graphics Synthesizer and SPU2 are vastly more capable. PS2 games rely on these; they cannot be "downgraded" to PS1's GPU/SPU.
What You Can Do Instead
Find the PS1 Version: Many franchises have distinct PS1 entries (e.g., Final Fantasy VII-IX, Metal Gear Solid, Crash Bandicoot trilogy). Buy original discs or check PSN Classics on PS3/PSP/Vita.
PS1 Emulation: Use DuckStation (Windows/Linux/macOS/Android), RetroArch (beetle-psx core), or ePSXe on PC/phone. Requires a legal BIOS dump and your own game ISOs.
PS2 Emulation: Play the PS2 ISO on PC via PCSX2 (now highly compatible) if your hardware supports it.
Legal Reminder: Emulation is legal; downloading ISOs/BIOS you don't own is copyright infringement.