Steam Achievements Don't Sync to Xbox 360 (Portal Example)
No. Steam (PC) and Xbox 360 (Xbox Live) are completely separate ecosystems. Achievements do not cross-platform.
Why
Different services: Steamworks vs. Xbox Live. No shared identity, no API bridge.
Different lists:Portal on Steam has ~30 achievements. Portal: Still Alive (XBLA) has 12 different ones. Portal 2 (Steam/PS3/Xbox 360) has platform-specific lists.
No account linking: Valve and Microsoft don't merge achievement data.
What You Can Do
Earn Steam achievements: Enjoy Portal on PC. They're tied to your Steam profile forever.
Buy the Xbox version:Portal: Still Alive (XBLA, delisted — need code/used account) or The Orange Box (disc, has Portal with 360 achievements).
Xbox One/Series:Portal not BC. Portal 2 is BC (via The Orange Box disc or digital if previously owned).
Cross-Platform Progression Exists For:
Fortnite, Rocket League, Destiny 2, CoD: Warzone, Minecraft (Bedrock), Apex Legends — via Epic/Activision/EA/Microsoft accounts.
Xbox Play Anywhere titles (buy once, play PC/Xbox, shared saves/achievements). Portal is not one.
Enjoy Portal on Steam. It's the definitive version (workshop mods, HD textures, commentary).