No. The Nintendo 64 Controller Pak (NUS-004) has fixed 256 KB (2 Mbit) EEPROM — not expandable. “Pages” refer to the 123-page directory structure (16 pages per save file max), but total capacity is hardware-limited.
Note: Controller Pak saves are distinct from cartridge saves (SRAM/FlashRAM/EEPROM on cart). Most single-player progress goes on cart; Pak used for multiplayer data, ghosts, photos, custom settings.