No. Physically and electrically incompatible.
| Console | Memory Format | Dimensions |
|---|---|---|
| PSP Go | Memory Stick Micro (M2) | 15 × 12.5 × 1.2 mm |
| PS Vita | PS Vita Memory Card (Proprietary) | 28 × 21 × 2.8 mm |
No adapter bridges M2 ↔ Vita card. Use M2 for PSP Go; Vita card for Vita.