No. Star Wars: The Force Unleashed (Xbox 360, PS3, PC, Wii, PS2, PSP, DS) is a **strictly single-player** action game. There is no cooperative, competitive, or online multiplayer mode in any version.
Star Wars: The Force Unleashed II (2010) is also **single-player only**.
If you want Star Wars multiplayer: Star Wars Battlefront (2004/2005), Battlefront II (2005/2017), Jedi Knight: Jedi Academy (PC/MP), SWTOR (MMO), Squadrons (MP dogfighting).